Electrostatic self‑assembly cellulose nanofibers/MXene/nickel chains for highly stable and efficient seawater evaporation and purification

서지정보

ㆍ발행기관 : 한국탄소학회 ㆍ수록지정보 : Carbon letters / 33권 / 7호
ㆍ저자명 : Shuai Yang, Cai Shi, Keqi Qu, Zhe Sun, Handong Li, Benbin Xu, Zhanhua Huang, Zhanhu Guo

목차

Electrostatic self-assembly cellulose nanofibersMXenenickel chains for highly stable and efficient seawater evaporation and purification
Abstract
Graphical abstract
1 Introduction
2 Experimental
2.1 Sample preparation
2.1.1 Preparation of MXene
2.1.2 Preparation of P-Ni chain
2.1.3 Preparation of CMN aerogel
2.2 Solar desalination test
3 Results and discussion
3.1 Characterization of CMNx
3.2 Solar-powered water evaporation performance of CMNX aerogels
4 Conclusion
Anchor 15
References

영어 초록

Seawater evaporation and purification powered by solar energy are considered as a promising approach to alleviate the global freshwater crisis, and the development of photothermal materials with high efficiency is imminent. In this study, cellulose nanofiber (CNF)/MXene/Ni chain (CMN) aerogels were successfully synthesized by electrostatic force and hydrogen bond interaction force. CMN10 achieved a favorable evaporation rate as high as 1.85 kg m− 2 h− 1 in pure water, and the corresponding evaporation efficiency could be up to 96.04%. Even if it is applied to seawater with multiple interference factors, its evaporation rate can still be 1.81 kg m− 2 h− 1. The superior seawater evaporation activity origins from the promoted separation of photoexcited charges and photothermal conversion by the synergy of Ni chain and MXene, as well as the water transport channel supported by the 3D structure frame of CNF. Most importantly, CMN aerogel can maintain water vapor evaporation rates above 1.73 kg m− 2 h− 1 under extreme conditions such as acidic (pH 2) and alkaline (pH 12) conditions. In addition, various major ions, heavy metals and organic pollutants in seawater can be rejected by CMN10 during desalination, and the rejection rates can reach more than 99.69%, ensuring the purity of water resources after treatment. This work shows the great potential of CMN aerogel as a high-efficiency solar evaporator and low-cost photothermal conversion material. Cellulose nanofiber (CNF)/MXene/Ni chain (CMN) aerogels demonstrated high evaporation of water from sea water.

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